• 文献标题:   Density of states deduced from ESR measurements on low-dimensional nanostructures; benchmarks to identify the ESR signals of graphene and SWCNTs
  • 文献类型:   Article
  • 作  者:   SZIRMAI P, FABIAN G, DORA B, KOLTAI J, ZOLYOMI V, KURTI J, NEMES NM, FORRO L, SIMON F
  • 作者关键词:   carbon nanotube, electron spin resonance, graphene, pauli susceptibility, spindecoherence, spintronic, spin lifetime
  • 出版物名称:   PHYSICA STATUS SOLIDI BBASIC SOLID STATE PHYSICS
  • ISSN:   0370-1972 EI 1521-3951
  • 通讯作者地址:   Budapest Univ Technol Econ
  • 被引频次:   12
  • DOI:   10.1002/pssb.201100191
  • 出版年:   2011

▎ 摘  要

Electron spin resonance (ESR) spectroscopy is an important tool to characterize the ground state of conduction electrons and to measure their spin-relaxation times. Observing ESR of the itinerant electrons is thus of great importance in graphene and in single-wall carbon nanotubes. Often, the identification of CESR signal is based on two facts: the apparent asymmetry of the ESR signal (known as a Dysonian lineshape) and on the temperature independence of the ESR signal intensity. We argue that these are insufficient as benchmarks and instead the ESR signal intensity (when calibrated against an intensity reference) yields an accurate characterization. We detail the method to obtain the density of states from an ESR signal, which can be compared with theoretical estimates. We demonstrate the success of the method for K doped graphite powder. We give a benchmark for the observation of ESR in graphene. (C) 2011 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim