• 文献标题:   Plasma-assisted facile fabrication of omniphobic graphene oxide membrane with anti-wetting property for membrane distillation
  • 文献类型:   Article
  • 作  者:   CHEN HM, MAO YY, MO BY, PAN Y, XU R, JI WQ, CHEN GN, LIU GP, JIN WQ
  • 作者关键词:   graphene oxide membrane, omniphobic membrane, plasma treatment, surface modification, membrane distillation
  • 出版物名称:   JOURNAL OF MEMBRANE SCIENCE
  • ISSN:   0376-7388 EI 1873-3123
  • 通讯作者地址:  
  • 被引频次:   0
  • DOI:   10.1016/j.memsci.2022.121207 EA NOV 2022
  • 出版年:   2023

▎ 摘  要

Novel design of omniphobic membrane could relieve the wetting phenomenon caused by low surface energy contaminants in the feed of membrane distillation process. In this work, we reported on a new kind of omni-phobic graphene oxide (GO) membrane fabricated by plasma treatment and subsequent fluoroalkyl grafting of stacked GO laminates. The plasma treatment not only created in-plane nanopores in GO nanosheets to provide more water channels, but also added active sites for fluoroalkyl grafting to build a robust omniphobic membrane surface. The resulting omniphobic membrane exhibited outperformed water flux of similar to 35 kg m-2 h(-1) and salt rejection of 99.9% for 35 g L-1 NaCl solution with 0.2-0.4 mM sodium dodecyl sulfate (SDS) at 60 degrees C during over 450 h of direct contact membrane distillation (DCMD) process. This work provides a facile strategy to develop high-flux and wetting-resistance materials for membrane distillation.