• 文献标题:   Liquid thin film dewetting-driven micropatterning of reduced graphene oxide electrodes for high performance OFETs
  • 文献类型:   Article
  • 作  者:   LEE SM, SONG SK, YOON S, CHUNG DS, CHANG ST
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF MATERIALS CHEMISTRY C
  • ISSN:   2050-7526 EI 2050-7534
  • 通讯作者地址:   Chung Ang Univ
  • 被引频次:   3
  • DOI:   10.1039/c8tc03981j
  • 出版年:   2019

▎ 摘  要

We present a novel approach to produce high-resolution reduced graphene oxide (rGO) micropatterns based on a dewetting phenomenon of liquid thin films. The uniform liquid thin film of aqueous graphene oxide (GO) dispersion was formed by the meniscus dragging deposition method on a pre-patterned silanized substrate. Subsequently, selective dewetting of the water layer was induced due to the surface energy gradient on the coating substrates. After drying and chemical reduction, the high-resolution rGO micropatterns with a minimum feature size of 10 m were realized over a large area substrate by consuming less than 1 L of GO solution per square centimeter. As a demonstration of the application of this patterning technique, we have successfully fabricated organic field-effect transistors (OFETs) based on rGO pattern arrays as source-drain electrodes. The OFETs with the rGO electrodes exhibited a field effect mobility of 0.6 cm(2) (V s)(-1) with an on/off ratio of 1.79 x 10(6), which is higher than that of the devices with Au source-drain contacts.