• 文献标题:   Correlated Topological States in Graphene Nanoribbon Heterostructures
  • 文献类型:   Article
  • 作  者:   JOOST JP, JAUHO AP, BONITZ M
  • 作者关键词:   graphene nanoribbon, heterostructure, topological state, electronic correlation, green function theory
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984 EI 1530-6992
  • 通讯作者地址:   Christian Albrechts Univ Kiel
  • 被引频次:   1
  • DOI:   10.1021/acs.nanolett.9b04075
  • 出版年:   2019

▎ 摘  要

Finite graphene nanoribbon (GNR) heterostructures host intriguing topological in-gap states (Rizzo, D. J.; et al. Nature 2018, 560, 204). These states may be localized either at the bulk edges or at the ends of the structure. Here we show that correlation effects (not included in previous density functional simulations) play a key role in these systems: they result in increased magnetic moments at the ribbon edges accompanied by a significant energy renormalization of the topological end states, even in the presence of a metallic substrate. Our computed results are in excellent agreement with the experiments. Furthermore, we discover a striking, novel mechanism that causes an energy splitting of the nonzero-energy topological end states for a weakly screened system. We predict that similar effects should be observable in other GNR heterostructures as well.