• 文献标题:   Graphene-mediated ferromagnetic coupling in the nickel nano-islands/graphene hybrid
  • 文献类型:   Article
  • 作  者:   GAO M, HAN XW, LIU WJ, TIAN ZA, MEI YF, ZHANG M, CHU P, KAN EJ, HU T, DU YP, QIAO S, DI ZF
  • 作者关键词:  
  • 出版物名称:   SCIENCE ADVANCES
  • ISSN:   2375-2548
  • 通讯作者地址:  
  • 被引频次:   5
  • DOI:   10.1126/sciadv.abg7054
  • 出版年:   2021

▎ 摘  要

Nanoscale magnetic structures are fundamental to the design and fabrication of spintronic devices and have exhibited tremendous potential superior to the conventional semiconductor devices. However, most of the magnetic moments in nanostructures are unstable due to size effect, and the possible solution based on exchange coupling between nanomagnetism is still not clear. Here, graphene-mediated exchange coupling between nanomagnets is demonstrated by depositing discrete superparamagnetic Ni nano-islands on single-crystal graphene. The heterostructure exhibits ideal two-dimensional (2D) ferromagnetism with clear hysteresis loops and Curie temperature up to 80 K. The intrinsic ferromagnetism in graphene and antiferromagnetic exchange coupling between graphene and Ni nano-islands are revealed by x-ray magnetic circular dichroism and density functional theory calculations. The artificial 2D ferromagnets constitute a platform to study the coupling mechanism between complex correlated electronic systems and magnetism on the nanoscale, and the results and concept provide insights into the realization of spin manipulation in quantum computing.