• 文献标题:   Lightweight graphene aerogels by decoration of 1D CoNi chains and CNTs to achieve ultra-wide microwave absorption
  • 文献类型:   Article
  • 作  者:   ZHAO B, LI Y, JI HY, BAI PW, WANG S, FAN BB, GUO XQ, ZHANG R
  • 作者关键词:   microwave absorption, magnetic graphene aerogel, 3d conductive network, ohmic los, polarization los
  • 出版物名称:   CARBON
  • ISSN:   0008-6223 EI 1873-3891
  • 通讯作者地址:  
  • 被引频次:   118
  • DOI:   10.1016/j.carbon.2021.01.136 EA FEB 2021
  • 出版年:   2021

▎ 摘  要

Hybrid aerogels combination of dielectric loss composition and magnetic loss constituent are supposed to be the appealing microwave absorption materials due to the synergy between dielectric and magnetic constituents, lightweight feature as well as multiple scattering. Herein, hybrid graphene aerogels with decoration of 1D CoNi chains and CNTs (GA-CNT-CoNi) were fabricated via a facile freeze-drying method and followed by thermal reduction. Compared with GA and GA-CoNi aerogels, 4 wt% GA-CNT-CoNi immersed in polydimethylsiloxane matrix reveals the strongest microwave absorption properties. The optimal reflection loss (RL) value is -50.8 dB at only thickness of 1.8 mm, and the effective absorption bandwidth (EAB, RL below -10 dB) can achieve 8.5 GHz (18-26.5 GHz) covering the whole K band. High ohmic loss induced by 3D macroscopic conductive network, multiple polarization as well as eddy current loss are responsible for the boosted microwave absorption. The results demonstrate that GA-CNT-CoNi aerogel reveals the characteristics of ultra-low filler content, strong absorption, ultra-wideband, small thickness and lightweight, which is considered as a promising microwave absorbing candidate. (C) 2021 Elsevier Ltd. All rights reserved.