• 文献标题:   Femtosecond carrier dynamics in bulk graphite and graphene paper
  • 文献类型:   Article
  • 作  者:   CARBONE F, AUBOCK G, CANNIZZO A, VAN MOURIK F, NAIR RR, GEIM AK, NOVOSELOV KS, CHERGUI M
  • 作者关键词:  
  • 出版物名称:   CHEMICAL PHYSICS LETTERS
  • ISSN:   0009-2614 EI 1873-4448
  • 通讯作者地址:   Ecole Polytech Fed Lausanne
  • 被引频次:   38
  • DOI:   10.1016/j.cplett.2011.01.052
  • 出版年:   2011

▎ 摘  要

Femtosecond white-light continuum probe transient absorption and reflectivity measurements of bulk graphite and graphene paper are reported. In graphite, the relaxation of photoinduced electron-hole pairs happens through in-plane electron-electron and electron-phonon scattering in similar or equal to 200 fs, while the ps dynamics is due to the modulation of the electronic structure by out-of-plane structural motions. The ps dynamics of the optical signal is strongly reduced in graphene paper, where the out-of-plane bond is disrupted, while the short component of the dynamics is identical in both materials. These results show that in 2D-graphene, the carrier relaxation occurs in similar or equal to 200 fs. (C) 2011 Elsevier B. V. All rights reserved.