• 文献标题:   One-pot synthesis of a ceria-graphene oxide composite for the efficient removal of arsenic species
  • 文献类型:   Article
  • 作  者:   SAKTHIVEL TS, DAS S, PRATT CJ, SEAL S
  • 作者关键词:  
  • 出版物名称:   NANOSCALE
  • ISSN:   2040-3364 EI 2040-3372
  • 通讯作者地址:   Univ Cent Florida
  • 被引频次:   13
  • DOI:   10.1039/c6nr07608d
  • 出版年:   2017

▎ 摘  要

Arsenic contamination has posed a health risk to millions of people around the world. In this study, we describe a simple and facile one-step hydrothermal synthesis of a ceria-graphene oxide (ceria-GO) composite for the efficient removal of arsenic species. The prepared ceria-GO composite materials exhibited almost complete (over 99.99%) and quick removal of both arsenic species within 0.1 mg L-1 of the initial concentration. The calculated adsorption capacities were 185 mg g(-1) for As(III) and 212 mg g(-1) for As(V). It was found that Ce3+ is an active site and continuously adsorbs arsenic species; there is a concomitant change from Ce4+ to Ce3+ due to the solution redox environment. This increase in the Ce3+ concentration further facilitates the complete removal of arsenic species in solution. Thus our approach offers a promising potential for the treatment of arsenic-contaminated drinking water.