• 文献标题:   Hybridized 1T/2H-MoS2/graphene fishnet tube for high-performance on-chip integrated micro-systems comprising supercapacitors and gas sensors
  • 文献类型:   Article
  • 作  者:   ZHANG C, NING J, WANG BY, GUO HB, FENG X, SHEN X, JIA YQ, DONG JG, WANG D, ZHANG JC, HAO Y
  • 作者关键词:   multifunctional system, integrate, 1t/2hmos2, supercapacitor, gas sensor
  • 出版物名称:   NANO RESEARCH
  • ISSN:   1998-0124 EI 1998-0000
  • 通讯作者地址:   Xidian Univ
  • 被引频次:   0
  • DOI:   10.1007/s12274-020-3052-x EA SEP 2020
  • 出版年:   2021

▎ 摘  要

The emerging micro-nano-processing technologies have propelled significant advances in multifunctional systems that can perform multiple functions within a small volume through integration. Herein, we present an on-chip multifunctional system based on a 1T/2H-MoS2/graphene fishnet tube, where a micro-supercapacitor and a gas sensor are integrated. A hybrid three-dimensional stereo nanostructure, including MoS(2)nanosheets and graphene fishnet tubes, provides K+ ions with a short diffusion pathway and more active sites. Owing to the large layer spacing of 1T-MoS(2)promoting fast reversible diffusion, the on-chip micro-supercapacitor exhibits excellent electrochemical properties, including an areal capacitance of 0.1 F center dot cm(-2)(1 mV center dot s(-1)). The variation in the conductivity of 2H-MoS2 when ammonia molecules are adsorbed as derived from the first-principles calculations proves the Fermi level-changes theory. Driven by a micro-supercapacitor, the responsivity of the gas sensor can reach 55.7% at room temperature (27 degrees C). The multifunctional system demonstrates the possibility of achieving a two-dimensional integrated system for wearable devices and wireless sensor networks in the future.