• 文献标题:   High performance Li-ion capacitor fabricated with dual graphene-based materials
  • 文献类型:   Article
  • 作  者:   SUI D, WU MM, LIU YY, YANG YL, ZHANG HT, MA YF, ZHANG L, CHEN YS
  • 作者关键词:   liion capacitor, rate capability, cycling stability, dual graphenebased material, energy density
  • 出版物名称:   NANOTECHNOLOGY
  • ISSN:   0957-4484 EI 1361-6528
  • 通讯作者地址:  
  • 被引频次:   30
  • DOI:   10.1088/1361-6528/abb9d8
  • 出版年:   2021

▎ 摘  要

Lithium-ion capacitors (LICs) are now drawing increasing attention because of their potential to overcome the current energy limitations of supercapacitors and power limitations of lithium-ion batteries. In this work, we designed LICs by combining an electric double-layer capacitor cathode and a lithium-ion battery anode. Both the cathode and anode are derived from graphene-modified phenolic resin with tunable porosity and microstructure. They exhibit high specific capacity, superior rate capability and good cycling stability. Benefiting from the graphene-enhanced electrode materials, the all graphene-based LICs demonstrate a high working voltage (4.2 V), high energy density of 142.9 Wh kg(-1), maximum power density of 12.1 kW kg(-1)with energy density of 50 Wh kg(-1), and long stable cycling performance (with similar to 88% capacity retention after 5000 cycles). Considering the high performance of the device, the cost-effective and facile preparation process of the active materials, this all graphene-based lithium-ion capacitor could have many promising applications in energy storage systems.