• 文献标题:   Functionally reduced graphene oxide supported iron oxides composites as an adsorbent for the immobilization of uranium ions from aqueous solutions
  • 文献类型:   Article
  • 作  者:   ZONG PF, CAO DL, CHENG Y, ZHANG HZ, SHAO DD, WANG SF, HE CH, ZHAO YL
  • 作者关键词:   mrgo, u vi, coexisted ligand, temperature, interaction mechanism
  • 出版物名称:   JOURNAL OF MOLECULAR LIQUIDS
  • ISSN:   0167-7322 EI 1873-3166
  • 通讯作者地址:   North Univ China
  • 被引频次:   5
  • DOI:   10.1016/j.molliq.2017.05.101
  • 出版年:   2017

▎ 摘  要

Comprehension the extent and rate of U(VI) adsorption on some mineral surfaces are significant to predict their migration and transformation properties in the environmental systems. Herein, iron oxides particles supported reduced graphene oxide composites (MRGO) were successfully synthesized by in-situ chemical precipitation approach. The MRGO composites which illustrated high saturation magnetization could be likely separated using an external magnet. The experimental data illustrated that U(VI) ions could be interacted with MRGO composites through different interaction mechanisms depending on different environmental conditions. The adsorption kinetic results can be well simulated using the pseudo-second-order pattern. The pH-dependent adsorption behavior illustrated an favorable pH value of 7.5 for removal of U(VI) ions using MRGO composites. Furthermore, the adsorption regeneration of MRGO composites in simulated wastewater disposal systems was tested. Based on above mentioned, it was clear that MRGO composites could be potentially used as adsorbent for removal of actual U(VI)-bearing wastewaters.(C) 2017 Elsevier B.V. All rights reserved.