• 文献标题:   Synthesis of silver phosphate/graphene oxide aerogel and its high visible light photocatalytic elimination of formaldehyde
  • 文献类型:   Article
  • 作  者:   ZHANG XY, LIU BR, YANG Y, LIU WB, HOU ZD, SHANG JW, CHENG XW
  • 作者关键词:   ag3po4/go, aerogel, visible light, formaldehyde, photocatalysi
  • 出版物名称:   JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
  • ISSN:   2213-2929 EI 2213-3437
  • 通讯作者地址:  
  • 被引频次:   4
  • DOI:   10.1016/j.jece.2022.107171 EA JAN 2022
  • 出版年:   2022

▎ 摘  要

For efficient degradation of volatile organic compounds (VOCs) in the air, promising and environmentally friendly technologies are being explored. Here, a silver phosphate/graphene oxide (Ag3PO4/GO) aerogel was synthesized by ultrasonic precipitation combined with freeze drying strategy. Afterwards, physicochemical properties of the as-obtained Ag3PO4/GO aerogel sample were investigated by scanning electron microscopy, transmission electron microscopy, X-ray diffraction, ultraviolet-visible diffuse reflectance spectroscopy, Raman spectroscopy, and X-ray photoelectron spectroscopy. Results showed that spherical Ag3PO4 with an average diameter of 150 nm uniformly combined with GO to form an aerogel structure. Moreover, by integrating with GO, the utilization rate, visible light absorption, and pollutant degradation efficiency of Ag3PO4 could be significantly improved. Furthermore, Ag3PO4/GO aerogel was used to degrade VOC (formaldehyde in this case), which was found to be degraded from 3.012 mg/m(3) to 0.419 mg/m(3) under a 180-minute Xenon lamp. Thus, the mechanism of enhanced visible light photocatalytic (PC) degradation of formaldehyde by Ag3PO4/GO aerogel was proposed and discussed. Finally, it provided a reference for the development prospects of environmentally friendly new materials to treat gaseous pollutants in the air.