• 文献标题:   Fabrication of a Ag3PO4/Reduced graphene oxide/BiOBr ternary photocatalyst for enhanced visible-light photocatalytic activity and stability
  • 文献类型:   Article
  • 作  者:   ZHANG R, HAN Q, LI Y, CAI YF, ZHANG TQ, LIU Y, ZHU XY
  • 作者关键词:   ag3po4/rgo/biobr, visiblelight, photocatalysi, dye degradation, mechanism
  • 出版物名称:   JOURNAL OF ALLOYS COMPOUNDS
  • ISSN:   0925-8388 EI 1873-4669
  • 通讯作者地址:   Southwest Petr Univ
  • 被引频次:   2
  • DOI:   10.1016/j.jallcom.2019.151868
  • 出版年:   2019

▎ 摘  要

In this work, a novel visible-light-driven photocatalyst Ag3PO4/RGO/BiOBr was successfully prepared with hydrothermal and precipitation methods. The morphology, structure and photocatalytic activity of the as-prepared photocatalyst were characterized by X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FT-IR), X-ray photoelectron spectroscopy (XPS), Scanning electron microscopy (SEM) and Transmission electron microscopy (TEM). The catalytic properties of photocatalysts were analysed by UV-Vis diffuse reflectance spectra (UV-Vis DRS). The degradation rate of methylene blue (MB) for the Ag3PO4/RGO/BiOBr composite (96.5%) was higher than that for BiOBr (60.25%), Ag3PO4 (68.27%) and Ag3PO4/BiOBr (84.96%) after visible light irradiation for 30 min. Moreover, a possible mechanism for the photocatalyst was proposed in this study, and the improvement of the photocatalytic performance was attributed to the effective separation and transfer of photostimulated electron-hole pairs. This catalytic mechanism is in agreement with photoluminescence spectra (PL), photoelectrochemical measurements and radical capture experiments. In general, the Ag3PO4/RGO/BiOBr photocatalyst has good application prospects for the degradation of dyes and environmental protection. (C) 2019 Elsevier B.V. All rights reserved.