• 文献标题:   Visible-Light Driven TiO2 Photocatalyst Coated with Graphene Quantum Dots of Tunable Nitrogen Doping
  • 文献类型:   Article
  • 作  者:   SUN X, LI HJ, OU NQ, LYU BW, GUI BJ, TIAN SW, QIAN DJ, WANG XY, YANG JH
  • 作者关键词:   ndoping gqd, titanium dioxide, surface modification, photocatalytic, rhb degradation
  • 出版物名称:   MOLECULES
  • ISSN:   1420-3049
  • 通讯作者地址:   Univ Shanghai Sci Technol
  • 被引频次:   9
  • DOI:   10.3390/molecules24020344
  • 出版年:   2019

▎ 摘  要

Nitrogen doped graphene quantum dots (NGQDs) were successfully prepared via a hydrothermal method using citric acid and urea as the carbon and nitrogen precursors, respectively. Due to different post-treatment processes, the obtained NGQDs with different surface modifications exhibited blue light emission, while their visible-light absorption was obviously different. To further understand the roles of nitrogen dopants and N-containing surface groups of NGQDs in the photocatalytic performance, their corresponding composites with TiO2 were utilized to degrade RhB solutions under visible-light irradiation. A series of characterization and photocatalytic performance tests were carried out, which demonstrated that NGQDs play a significant role in enhancing visible-light driven photocatalytic activity and the carrier separation process. The enhanced photocatalytic activity of the NGQDs/TiO2 composites can possibly be attributed to an enhanced visible light absorption ability, and an improved separation and transfer rate of photogenerated carriers.