• 文献标题:   Angle-Resolved Photoemission Spectra of Graphene from First-Principles Calculations
  • 文献类型:   Article
  • 作  者:   PARK CH, GIUSTINO F, SPATARU CD, COHEN ML, LOUIE SG
  • 作者关键词:  
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984 EI 1530-6992
  • 通讯作者地址:   Univ Calif Berkeley
  • 被引频次:   81
  • DOI:   10.1021/nl902448v
  • 出版年:   2009

▎ 摘  要

Angle-resolved photoemission spectroscopy (ARPES) is a powerful experimental technique for directly probing electron dynamics in solids. The energy versus momentum dispersion relations and the associated spectral broadenings measured by ARPES provide a wealth of information on quantum many-body interaction effects. In particular, ARPES allows studies of the Coulomb interaction among electrons (electron-electron interactions) and the interaction between electrons and lattice vibrations (electron-phonon interactions). Here, we report ab initio simulations of the ARPES spectra of graphene including both electron-electron and electron-phonon interactions on the same footing. Our calculations reproduce some of the key experimental observations related to many-body effects, including the indication of a mismatch between the upper and lower halves of the Dirac cone.