• 文献标题:   Broadband optical response of graphene measured by terahertz time-domain spectroscopy and FTIR spectroscopy
  • 文献类型:   Article
  • 作  者:   ARTS K, VERVUURT R, BHATTACHARYA A, RIVAS JG, OOSTERBEEK JW, BOL AA
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF APPLIED PHYSICS
  • ISSN:   0021-8979 EI 1089-7550
  • 通讯作者地址:   Eindhoven Univ Technol
  • 被引频次:   3
  • DOI:   10.1063/1.5044265
  • 出版年:   2018

▎ 摘  要

This work describes the broadband optical response of graphene grown by chemical vapor deposition by combining terahertz time-domain spectroscopy (THz-TDS) at 0.25-1.7 THz (8-60cm(-1)) with Fourier Transform Infrared Spectroscopy (FTIR) at 11-210 THz (370-7000cm(-1)). It is shown that the measured response is well described by a combination of the Drude model, expressing freecarrier absorption/reflection, and an expression for interband absorption. The THz-TDS and FTIR transmittance curves are fitted consistently using this model. This indicates that these techniques are complementary to each other. Both can thus be employed together or individually to characterize the electronic properties of graphene (e.g., carrier density and mobility). To exemplify this, we demonstrate that this equivalency can be used to study the effect of substrate-dependent doping on the optical response of graphene. Furthermore, the amount of reflection and absorption corresponding to the measured transmittance curve is calculated. The toolbox for the non-invasive broadband characterization of graphene is thus extended by this work. Published by AIP Publishing.