• 文献标题:   Development of Broadband PbS Quantum Dot/Graphene Photodetector Arrays with High-Speed Readout Circuits for Flexible Imagers
  • 文献类型:   Article
  • 作  者:   SHULTZ A, LIU B, GONG MG, ALAMRI M, WALSH M, SCHMITZ RC, WU JZ
  • 作者关键词:   quantum dot, graphene, nanohybrid photodetector, flexible, broadband imaging array
  • 出版物名称:   ACS APPLIED NANO MATERIALS
  • ISSN:  
  • 通讯作者地址:  
  • 被引频次:   3
  • DOI:   10.1021/acsanm.2c03839 EA NOV 2022
  • 出版年:   2022

▎ 摘  要

Colloidal quantum dot (QD)/graphene nanohybrid heterostructures provide a promising scheme for quantum sensors as they take advantage of the strong quantum confinement in QDs with enhanced light-matter interaction, spectral tunability, suppressed phonon scattering, and extraordinary charge mobility in graphene at room temperature. Herein, we report development of a flexible, nine-channel PbS QD/graphene nanohybrid imaging array on polyethylene terephthalate using a facile process for device fabrication, signal acquisition, and processing. The PbS QD/graphene imaging array exhibited high and uniform photoresponse. At a 1.0 V bias, the highest responsivity was 9.56 X 10(3)-3.24 X 10(3) A/W for 400-1000 nm incident light [ultraviolet-visible-near-infrared (UV-vis-NIR)] with a power of 900 pW. In addition, the array has a consistent spectral response with bending down to a radius of curvature of a few millimeters. The demonstration of imaging at broadband wavelengths in the UV-vis-NIR range indicates that QD/graphene nanohybrids provide a viable approach for flexible photodetectors and imagers.