• 文献标题:   Direct Printing of Graphene Electrodes for High-Performance Organic Inverters
  • 文献类型:   Article
  • 作  者:   NAIK AR, KIM JJ, USLUER O, ARELLANO DLG, SECOR EB, FACCHETTI A, HERSAM MC, BRISENO AL, WATKINS JJ
  • 作者关键词:   direct transfer printing, graphene ink, organic transistor, graphene pattern, printed electronic
  • 出版物名称:   ACS APPLIED MATERIALS INTERFACES
  • ISSN:   1944-8244
  • 通讯作者地址:   Univ Massachusetts
  • 被引频次:   5
  • DOI:   10.1021/acsami.8b01302
  • 出版年:   2018

▎ 摘  要

Scalable fabrication of high-resolution electrodes and interconnects is necessary to enable advanced, high-performance, printed, and flexible electronics. Here, we demonstrate the direct printing of graphene patterns with feature widths from 300 mu m to similar to 310 nm by liquid-bridge-mediated nanotransfer molding. This solution-based technique enables residue-free printing of graphene patterns on a variety of substrates with surface energies between similar to 43 and 73 mN m(-1). Using printed graphene source and drain electrodes, high-performance organic field-effect transistors (OFETs) are fabricated with single-crystal rubrene (p-type) and fluorocarbon-substituted dicyanoperylene-3,4:9,10-bis(dicarboximide) (PDIF-CN2) (n-type) semiconductors. Measured mobilities range from 2.1 to 0.2 cm(2) V-1 s(-1) for rubrene and from 0.6 to 0.1 cm(2) V-1 s(-1) for PDIF-CN2. Complementary inverter circuits are fabricated from these single-crystal OFETs with gains as high as, 50. Finally, these high-resolution graphene patterns are compatible with scalable processing, offering compelling opportunities for inexpensive printed electronics with increased performance and integration density.