▎ 摘　　要

3D graphene-based materials are promising adsorbents for environmental applications. Furthermore, increasing attention has been paid to the improvement of 3D graphene adsorbents for removing pollutants. In this article, the progress in the modification of 3D graphene materials and their performance for removing pollutants were reviewed. The modification strategies, which were classified as (1) the activation with CO2 (steam and other oxidants) and (2) the surface functionalization with polymers (metals, and metal oxides), were evaluated. The performances of modified 3D graphene materials were assessed for the removal of waste gases (such as CO2), refractory organics, and heavy metals. The challenges and future research directions were discussed for the environmental applications of 3D graphene materials. (C) 2020 Elsevier Ltd. All rights reserved.