• 文献标题:   Thermal Transport in Multidimensional Silicon-Graphene Hybrid Nanostructures
  • 文献类型:   Article
  • 作  者:   GONG W, GARG R, GUO RQ, LEE S, COHENKARNI T, SHEN S
  • 作者关键词:   multidimensional silicongraphene hybrid nanowire, 3d graphene flake, thermal conductivity
  • 出版物名称:   ACS APPLIED MATERIALS INTERFACES
  • ISSN:   1944-8244 EI 1944-8252
  • 通讯作者地址:  
  • 被引频次:   2
  • DOI:   10.1021/acsami.1c08093 EA OCT 2021
  • 出版年:   2021

▎ 摘  要

In this work, we fabricate multidimensional silicon-graphene hybrid nanostructures composed of three-dimensional (3D) out-of-plane graphene flakes on a silicon nanowire core. By changing the synthesis temperature (700 and 1100 degrees C) and time (5, 10, and 20 min), we obtain two different types of 3D graphene flakes with tunable dimensions and structure parameters. We characterize the thermal transport behavior of this hybrid multidimensional material in a broad temperature range of 20-460 K. With different morphologies and structures, the effective thermal conductivity of the silicon-graphene hybrid nanostructures varies from 1 to 7 W/(m.K) at room temperature. We also apply molecular dynamics simulation and density functional theory to elucidate the thermal transport mechanisms in the silicon-graphene hybrid nanostructures.