• 文献标题:   Giant quasiparticle bandgap modulation in graphene nanoribbons supported on weakly interacting surfaces
  • 文献类型:   Article
  • 作  者:   JIANG XP, KHARCHE N, KOHL P, BOYKIN TB, KLIMECK G, LUISIER M, AJAYAN PM, NAYAK SK
  • 作者关键词:  
  • 出版物名称:   APPLIED PHYSICS LETTERS
  • ISSN:   0003-6951 EI 1077-3118
  • 通讯作者地址:   Rensselaer Polytech Inst
  • 被引频次:   21
  • DOI:   10.1063/1.4822427
  • 出版年:   2013

▎ 摘  要

In general, there are two major factors affecting bandgaps in nanostructures: (i) the enhanced electron-electron interactions due to confinement and (ii) the modified self-energy of electrons due to the dielectric screening. While recent theoretical studies on graphene nanoribbons (GNRs) report on the first effect, the effect of dielectric screening from the surrounding materials such as substrates has not been thoroughly investigated. Using large-scale electronic structure calculations based on the GW approach, we show that when GNRs are deposited on substrates, bandgaps get strongly suppressed (by as much as 1 eV) even though the GNR-substrate interaction is weak. (C) 2013 AIP Publishing LLC.