• 文献标题:   Contamination-induced inhomogeneity of noise sources distribution in Al2O3-passivated quasi-free-standing graphene on 4H-SiC(0001)
  • 文献类型:   Article
  • 作  者:   CIUK T, CIURA L, MICHALOWSKI PP, JAGIELLO J, DOBROWOLSKI A, PIETAK K, KALITA D, WZOREK M, BUDZICH R, CZOLAK D, KOLEK A
  • 作者关键词:   graphene, silicon carbide, atomic layer deposition, aluminum oxide, noise measurement, contamination
  • 出版物名称:   PHYSICA ELOWDIMENSIONAL SYSTEMS NANOSTRUCTURES
  • ISSN:   1386-9477 EI 1873-1759
  • 通讯作者地址:  
  • 被引频次:   3
  • DOI:   10.1016/j.physe.2022.115264 EA APR 2022
  • 出版年:   2022

▎ 摘  要

In this report, we introduce a novel method based on low-frequency noise analysis for the assessment of quality and pattern of inhomogeneity in intentionally-aged Hall effect sensors featuring hydrogen-intercalated quasi-free-standing epitaxial Chemical Vapor Deposition graphene mesa on semi-insulating high-purity on -axis 4H-SiC(0001), all passivated with a 100-nm-thick atomic-layer-deposited Al(2)O(3)layer. Inferring from the comparison of the measured noise and one calculated for a homogeneous sensor, we hypothesize about possible unintentional contamination of the sensors' active regions. Following in-depth structural characterization based on Nomarski interference contrast optical imaging, confocal micro-Raman spectroscopy, high-resolution Transmission Electron Microscopy and Secondary Ion Mass Spectrometry, we find out that the graphene's quasi-free-standing character and p-type conductance make the Al2O3/graphene interface exceptionally vulnerable to uncontrolled contamination and its unrestrained lateral migration throughout the entire graphene mesa, eventually leading to the blistering of Al2O3. Thus, we prove the method's suitability for the detection of these contaminants' presence and location, and infer on its applicability to the investigation of any contamination-induced inhomogeneity in two-dimensional systems.