• 文献标题:   Enhancing Thermoelectric Properties of 2D Bi2Se3 by 1D Texturing with Graphene
  • 文献类型:   Article
  • 作  者:   WU JK, HOFMANN M, HSIEH WP, CHEN SH, YEN ZL, CHIU SK, LUO YR, CHIANG CC, HUANG SY, CHANG YH, HSIEH YP
  • 作者关键词:   thermoelectric, twodimensional, bi2se3, graphene, thermal conductivity, high zt
  • 出版物名称:   ACS APPLIED ENERGY MATERIALS
  • ISSN:   2574-0962
  • 通讯作者地址:   Natl Taiwan Univ
  • 被引频次:   1
  • DOI:   10.1021/acsaem.9b02122
  • 出版年:   2019

▎ 摘  要

Two-dimensional (2D) thermoelectrics have shown enhanced performance compared to bulk thermoelectrics but cannot easily be improved through nanostructuring, since phonon-boundary-scattering becomes ineffective under confined dimensions. To overcome this issue, we introduce a one-dimensional (ID) texturing approach that efficiently suppresses phonon transport between grains of 2D thermoelectrics (TE). Uniaxial graphene wrinkles were utilized to separate high-quality, ultrathin Bi2Se3 films in a highly directional manner. The TE properties of these textured samples exhibit a strongly anisotropic characteristic with a maximum ZT of 1.03 at room temperature, which represents the highest reported value for Bi2Se3. The texturing approach provides a route for the enhancement of 2D thermoelectrics for future applications.