• 文献标题:   Scalable Holey Graphene Synthesis and Dense Electrode Fabrication toward High-Performance Ultracapacitors
  • 文献类型:   Article
  • 作  者:   HAN XG, FUNK MR, SHEN F, CHEN YC, LI YY, CAMPBELL CJ, DAI JQ, YANG XF, KIM JW, LIAO YL, CONNELL JW, BARONE V, CHEN ZF, LIN Y, HU LB
  • 作者关键词:   scalable synthesi, facile processability, holey graphene, dense graphene electrode, ultracapacitor, supercapacitor, volumetric capacitance
  • 出版物名称:   ACS NANO
  • ISSN:   1936-0851 EI 1936-086X
  • 通讯作者地址:   Coll William Mary
  • 被引频次:   117
  • DOI:   10.1021/nn502635y
  • 出版年:   2014

▎ 摘  要

Graphene has attracted a lot of attention for ultracapacitor electrodes because of its high electrical conductivity, high surface area and superb chemical stability. However, poor volumetric capacitive performance of typical graphene-based electrodes has hindered their practical applications because of the extremely low density. Herein we report a scalable synthesis method of holey graphene (h-Graphene) in a single step without using any catalysts or special chemicals The film made of the as synthesized h-Graphene exhibited relatively strong mechanical strength, 2D hole morphology, high density, and facile processability. This scalable one-step synthesis method for h-Graphene is time environmentally friendly, and generally applicable to other two-dimensional materials The ultracapacitor electrodes based on remarkably improved volumetric capacitance with about 700% increase compared to that of regular graphene electrodes. h-Graphene was carried out to understand the excellent processability and improved ultracapacitor performance. efficient, the h-Graphene show a Modeling on individual cost-efficient,