• 文献标题:   Strain-Induced Plasmon Confinement in Polycrystalline Graphene
  • 文献类型:   Article
  • 作  者:   ZANOTTO S, BONATTI L, PANTANO MF, MISEIKIS V, SPERANZA G, GIOVANNINI T, COLETTI C, CAPPELLI C, TREDICUCCI A, TONCELLI A
  • 作者关键词:   graphene, terahertz, plasmon, strain, drudesmith, conductivity of polycrystalline 2d material, atomistic simulation
  • 出版物名称:   ACS PHOTONICS
  • ISSN:   2330-4022
  • 通讯作者地址:  
  • 被引频次:   1
  • DOI:   10.1021/acsphotonics.2c01157 EA JAN 2023
  • 出版年:   2023

▎ 摘  要

Terahertz spectroscopy is a perfect tool to investigate the electronic intraband conductivity of graphene, but a phenom-enological model (Drude-Smith) is often needed to describe disorder. By studying the THz response of isotropically strained polycrystalline graphene and using a fully atomistic computational approach to fit the results, we demonstrate here the connection between the Drude-Smith parameters and the microscopic behavior. Importantly, we clearly show that the strain-induced changes in the conductivity originate mainly from the increased separation between the single-crystal grains, leading to enchanced localization of the plasmon excitations. Only at the lowest strain values explored, a behavior consistent with the deformation of the individual grains can instead be observed.