• 文献标题:   Enhanced charge extraction for all-inorganic perovskite solar cells by graphene oxide quantum dots modified TiO2 layer
  • 文献类型:   Article
  • 作  者:   LIU YL, CHE GL, CUI WZ, PANG BL, SUN Q, YU LY, DONG LF
  • 作者关键词:   all inorganic, perovskite solar cell, graphene oxide quantum dot, high performance, stability
  • 出版物名称:   FRONTIERS OF CHEMICAL SCIENCE ENGINEERING
  • ISSN:   2095-0179 EI 2095-0187
  • 通讯作者地址:  
  • 被引频次:   0
  • DOI:   10.1007/s11705-022-2238-z EA FEB 2023
  • 出版年:   2023

▎ 摘  要

All-inorganic cesium lead bromide (CsPbBr3) perovskite solar cells have been attracting growing interest due to superior performance stability and low cost. However, low light absorbance and large charge recombination at TiO2/CsPbBr3 interface or within CsPbBr3 film still prevent further performance improvement. Herein, we report devices with high power conversion efficiency (9.16%) by introducing graphene oxide quantum dots (GOQDs) between TiO2 and perovskite layers. The recombination of interfacial radiation can be effectively restrained due to enhanced charge transfer capability. GOQDs with C-rich active sites can involve in crystallization and fill within the CsPbBr3 perovskite film as functional semiconductor additives. This work provides a promising strategy to optimize the crystallization process and boost charge extraction at the surface/interface optoelectronic properties of perovskites for high efficient and low-cost solar cells.