• 文献标题:   Simulated sunlight photodegradation of aqueous atrazine and rhodamine B catalyzed by the ordered mesoporous graphene-titania/silica composite material
  • 文献类型:   Article
  • 作  者:   LI KX, HUANG Y, YAN LS, DAI YH, XUE KP, GUO HQ, HUANG ZM, XIONG JJ
  • 作者关键词:   heterogeneous photocatalysi, graphene, titania, silica, ordered mesoporous material
  • 出版物名称:   CATALYSIS COMMUNICATIONS
  • ISSN:   1566-7367 EI 1873-3905
  • 通讯作者地址:   Nanchang Hangkong Univ
  • 被引频次:   22
  • DOI:   10.1016/j.catcom.2011.11.008
  • 出版年:   2012

▎ 摘  要

Ordered mesoporous graphene-titania/silica composite material was prepared using a direct sol-gel co-condensation technique, and combined with hydrothermal treatment, in the presence of a triblock copolymer non-ionic surfactant P123 (EO20PO70EO20. EO= -OCH2CH2-, PO= -OCH(CH3)CH2-). The composite exhibited a two-dimensional (2D) hexagonal p6mm symmetry and anatase-phase structure with a large BET (Brunauer-Emmet-Teller) surface area and uniform pore size. The photocatalytic activity of the graphene-titania/silica composite was evaluated through the degradation of the aqueous organic pollutant atrazine and rhodamine B under solar-simulating Xe lamp irradiation. Enhanced photocatalytic activity compared with pure titania was obtained for the graphene-titania/silica sample. (C) 2011 Elsevier B.V. All rights reserved.