• 文献标题:   Flexibility of Key Electronic and Optical Properties of Reduced Graphene Oxide Through Its Controlled Synthesis
  • 文献类型:   Article
  • 作  者:   NARZARY R, PHUKAN P, DAS S, SAHU PP
  • 作者关键词:   bandgap tuning, carrier concentration, deoxygenation, mobility, nanocomposite, nanostructure, reduced graphene oxide rgo
  • 出版物名称:   IEEE TRANSACTIONS ON ELECTRON DEVICES
  • ISSN:   0018-9383 EI 1557-9646
  • 通讯作者地址:  
  • 被引频次:   0
  • DOI:   10.1109/TED.2022.3204735 EA SEP 2022
  • 出版年:   2022

▎ 摘  要

Recently, graphene oxides (GOs), reduced GO (rGO), and their derivatives have been focused on as a superior flexible material due to having easy processability and high carrier mobility. Here, we report an inexpensive green synthesis of GO/rGO at a relatively low temperature of 150 degrees C. The scanning electron microscopy (SEM)/energy-dispersive X-ray (EDX), X-ray diffraction (XRD), Raman, Fourier transformed IR (FTIR), and UV-visible spectroscopy confirm the successful fabrication of rGO with an enhanced carbon-0carbon (sp(2)/sp(3)) component with an enhanced carbon-to-oxygen ratio (C/O) from 0.93 to 2.76. Here, a work function tuning of 5.6-4.5 eV, a bandgap modulation of 3.93-2.63 eV, a charge carrier density tuningfrom 1.12 x 10(16) to 1.14 x 10(21) cm(-3), and a mobility tuning from 1.51 x 10(-2) to 59.663 cm(2)/V.s are made through its controlled reduction of GOs, which are much better than the results obtained at high temperature >1000 degrees C. The flexible nature of both electronic and optical properties of rGO nanostructures assures it as an excellent material for electronics and optoelectronics devices.