• 文献标题:   Coherent Detection of Terahertz Radiation with Graphene
  • 文献类型:   Article
  • 作  者:   OBRAZTSOV PA, CHIZHOV PA, KAPLAS T, BUKIN VV, SILVENNOINEN M, HSIEH CF, KONISHI K, NEMOTO N, KUWATAGONOKAMI M
  • 作者关键词:   graphene, terahertz detector, timedomain terahertz spectroscopy, photoconductivity, hot carrier
  • 出版物名称:   ACS PHOTONICS
  • ISSN:   2330-4022
  • 通讯作者地址:   Russian Acad Sci
  • 被引频次:   3
  • DOI:   10.1021/acsphotonics.9b00536
  • 出版年:   2019

▎ 摘  要

Despite that significant efforts have been made in the development of time-integrated graphene-based detectors operating in vis/IR/THz ranges, little is known about coherent detection of THz pulses with graphene. To date only a few time resolved studies with on-chip detection schemes, which significantly limit the spectral range naturally provided by the gapless band structure of graphene, are known. Here we demonstrate free-space room-temperature detection of THz radiation in a wide spectral range with optically gated graphene. The detection principle is based on registration of the time-domain waveform of the THz field by measuring the hot-carrier photocurrent under THz pulse exposure in optically excited graphene using a pump probe scheme. The applied method is simple and robust, while the sensitivity and working range of the developed graphene-based detector are comparable and in some aspects outperform materials conventionally used for terahertz time domain spectroscopy based on electro-optic sampling and photoconductive antennas. In addition, we demonstrate that efficient coherent detection of terahertz radiation in a wide range to above 2 THz does not require highly crystalline, single-layer graphene but can be also realized with ultrathin graphite film, which is synthesized directly on an arbitrary dielectric substrate. Employment of such a material for fabrication of ultrafast terahertz detectors creates a versatile platform for the scalable production of wide-aperture photoconductive detectors applicable in spatially resolved time-domain terahertz spectrometers and visualizers.