• 专利标题:   Preparing silicon/amorphous carbon/graphene lithium ion battery anode material by mixing ethyl orthosilicate and alkaline catalyst, drying, mixing magnesium powder and heat removal agent, heating, adding glucose, graphene oxide and heating.
  • 专利号:   CN111106338-A
  • 发明人:   WANG Y, GUO X, YANG H, WANG J
  • 专利权人:   UNIV ZHEJIANG
  • 国际专利分类:   H01M010/0525, H01M004/38, H01M004/62
  • 专利详细信息:   CN111106338-A 05 May 2020 H01M-004/38 202042 Pages: 10 Chinese
  • 申请详细信息:   CN111106338-A CN11364473 26 Dec 2019
  • 优先权号:   CN11364473

▎ 摘  要

NOVELTY - Preparing silicon/amorphous carbon/graphene lithium ion battery anode material involves (i) mixing ethyl orthosilicate, alkaline catalyst and deionized water, magnetically stirring for 3 plus minus 0.3 hours, and performing centrifugal drying to obtain nano-silica particles, mixing nano-silica particles and magnesium powder, adding heat removal agent, heating at 650 plus minus 50 degrees C under inert gas and heat-preserving for 3 plus minus 0.3 hours to obtain nano-silicon particles, adding silicon nanoparticles and glucose to deionized water, stirring at 60 plus minus 10 degrees C for 5 plus minus 0.5 hours, and heating at 550 plus minus 50 degrees C under an inert gas to maintain for 3 plus minus 0.3 hours to obtain carbon-coated nano-silicon particles, and (ii) mixing carbon-coated nano-silicon particles with graphene oxide, adding deionized water, stirring for 12 plus minus 1 hours, freeze-drying, heating at 300 plus minus 50 degrees C under inert gas to maintain for 1 plus minus 0.1 hours and heating at 900 plus minus 50 degrees C to maintain for 2 plus minus 0.2 hours to obtain the product. USE - The method is useful for preparing silicon/amorphous carbon/graphene lithium ion battery anode material. DETAILED DESCRIPTION - Method for preparing silicon/amorphous carbon/graphene lithium ion battery anode material involves (i) mixing ethyl orthosilicate, alkaline catalyst and deionized water in a volume ratio of 1:(2 plus minus 0.2):(7 plus minus 0.5), magnetically stirring for 3 plus minus 0.3 hours, and performing centrifugal drying to obtain nano-silica particles, mixing nano-silica particles and magnesium powder in a weight ratio of 8:(7 plus minus 0.5), adding heat removal agent, heating at 650 plus minus 50 degrees C under inert gas and heat-preserving for 3 plus minus 0.3 hours to obtain nano-silicon particles, adding silicon nanoparticles and glucose to deionized water in a weight ratio of 1:(10 plus minus 1), stirring at 60 plus minus 10 degrees C for 5 plus minus 0.5 hours, and heating at 550 plus minus 50 degrees C under an inert gas to maintain for 3 plus minus 0.3 hours to obtain carbon-coated nano-silicon particles, and (ii) mixing carbon-coated nano-silicon particles with graphene oxide in a weight ratio of 1:(6 plus minus 0.5), adding deionized water, stirring for 12 plus minus 1 hours, freeze-drying, heating at 300 plus minus 50 degrees C under inert gas to maintain for 1 plus minus 0.1 hours and heating at 900 plus minus 50 degrees C to maintain for 2 plus minus 0.2 hours to obtain the product.