▎ 摘　　要

NOVELTY - Preparation of three-dimensional structure of graphene aerogels comprises obtaining mold, injecting functional material ink into the mold, freeze forming, transfer printing to obtain first ice layer, repeating steps, transferring layers of ice layer by layer on first layer and drying. The layer of functional material ink comprises graphene oxide and/or graphene. USE - The method is for preparation of three-dimensional structure of graphene aerogels. ADVANTAGE - The method is simple, efficient and conducive to large-scale fabrication of graphene aerogels.