▎ 摘　　要

NOVELTY - Performing integration of vertically aligned carbon nanotubes into graphene as three-dimensional structure involves preparing a colloid mixture of carbon nano tube (CNT) and reduced graphene oxide (RGO) by adding CNT and RGO separately in a suitable solvent. The colloidal mixtures sonicated separately in order to provide better dispersion in the solvent facilitating proper alignment and interaction. The CNT colloidal mixture placed between the electrodes in the glass container. A direct current (DC) electric field between the electrodes, caused aligning of the CNTs along the direction of the field. The RGO colloid mixture added to the aligned CNT composite slowly under continuous application of electric field causing the interaction between the CNT and the defect sites on RGO forming a nanohybrid. The nanohybrid is thermal dried for 24 hours. USE - Method for performing integration of vertically aligned carbon nanotubes into graphene as three-dimensional structure. ADVANTAGE - The method provides a simple and versatile method of intercalating CNT between graphene oxide to prepare CNT aligned between graphene as three dimensional (3D) nanocomposite by applying a DC electric field, which provide significant properties advantages over individual ones in applications.