• 专利标题:   Preparing graphene-carbon nanotube composite adsorbent, which is used to remove aqueous solution of tetracycline, involves weighing graphene oxide solution and ultrasonically stripping to obtain graphene oxide.
  • 专利号:   CN105642236-A
  • 发明人:   HAN S, LI Y, WANG J, YU F, SUN S
  • 专利权人:   SHANGHAI INST TECHNOLOGY
  • 国际专利分类:   B01J020/22, B01J020/28, C02F001/28, C02F101/30
  • 专利详细信息:   CN105642236-A 08 Jun 2016 B01J-020/22 201659 Pages: 5 Chinese
  • 申请详细信息:   CN105642236-A CN10075111 03 Feb 2016
  • 优先权号:   CN10075111

▎ 摘  要

NOVELTY - The preparation method of graphene-carbon nanotube composite adsorbent involves: (1) weighing 2 mg/ml graphene oxide solution and ultrasonically stripping to obtain graphene oxide; (2) adding certain amount of ascorbic acid to above solution and carrying out ultrasonic treatment for certain period of time; (3) mixing carbon nanotubes with 10 ml deionized water and resulting solution obtained in step (2), carrying out ultrasonic treatment for 2 hours and again carrying out ultrasonic treatment 0.5-1 hour; and (4) transferring the resulting mixture obtained in step (3) to beaker. USE - The method is useful for preparing graphene-carbon nanotube composite adsorbent, which is useful for removing aqueous solution of tetracycline. ADVANTAGE - The method enables simple and economical preparation of graphene-carbon nanotube composite adsorbent with high yield. DETAILED DESCRIPTION - The preparation method of graphene-carbon nanotube composite adsorbent involves: (1) weighing 2 mg/ml graphene oxide solution and ultrasonically stripping to obtain graphene oxide; (2) adding certain amount of ascorbic acid to above solution and carrying out ultrasonic treatment for certain period of time; (3) mixing carbon nanotubes with 10 ml deionized water and resulting solution obtained in step (2), carrying out ultrasonic treatment for 2 hours and again carrying out ultrasonic treatment for 0.5-1 hour; and (4) transferring the resulting mixture obtained in step (3) to beaker, carrying out reaction under water bath at 80 degrees C for 10-14 hours, then immersing resulting material in deionized water to obtain graphene-carbon nanotubes composite hydrogel and carrying out freeze-drying.