▎ 摘　　要

NOVELTY - The invention discloses a method of manufacturing ordered arrangement of graphene-carbon nano tube of metal substrate and composite coatings for carbon deposit, which deposits sputtering target and penetrating fluid into evacuated penetrating oven in order to make the penetrating fluid penetrates the sputtering target in the evacuated penetrating oven, and places the penetrated sputtering target into evacuated magnetic control sputtering machine and controls cooling water of the evacuated magnetic control sputtering target machine, namely, operates evacuated magnetic control sputtering process on the metal substrate, utilizes the characteristic of metal organic salt of the penetrating fluid that can remain non-magnetic under 150℃before decomposition, decomposes nano metal organic salt particles in high temperature zone after being sputtering and depositing on the metal substrate as catalyst of carbon so the carbon that came from the sputtering target can form carbon structural layer on concave / convex rough portion of the metal substrate. Accordingly, the invention reflects the beneficial effects of being easy and time saving on manufacture.