• 专利标题:   Preparing graphene material using Plumeria rubra as raw material by crushing dried Plumeria rubra, subjecting crushed Plumeria rubra to nitrogen atmosphere conditions, then putting into tubular furnace, heating, and heat preserving.
  • 专利号:   CN107381547-A
  • 发明人:   ZENG H, ZENG G, WANG Y
  • 专利权人:   UNIV SOUTH CHINA TECHNOLOGY
  • 国际专利分类:   C01B032/184
  • 专利详细信息:   CN107381547-A 24 Nov 2017 C01B-032/184 201801 Pages: 8 Chinese
  • 申请详细信息:   CN107381547-A CN10625161 27 Jul 2017
  • 优先权号:   CN10625161

▎ 摘  要

NOVELTY - The preparation method of graphene material using Plumeria rubra as raw material involves: (1) crushing dried P.rubra; (2) subjecting P.rubra obtained in step (1) to nitrogen atmosphere conditions, then putting into tubular furnace, heating, carrying out heat preservation, continuously heating at 800-950 degrees C, carrying out heat preservation for 1-2 hours, and slowly cooling to obtain pre-carbonized product; and (3) mixing the pre-carbonized product obtained in step (2) with activating agent, and then placing in tubular furnace under nitrogen atmosphere. USE - The method is useful for preparing graphene material using P.rubra as raw material (claimed). ADVANTAGE - The method enables simple, safe and economical preparation of graphene material using P.rubra as raw material with high yield in an environmentally-friendly manner. DETAILED DESCRIPTION - The preparation method of graphene material using Plumeria rubra as raw material involves: (1) crushing dried P.rubra; (2) subjecting P.rubra obtained in step (1) to nitrogen atmosphere conditions, then putting into tubular furnace, heating at 450-500 degrees C, carrying out heat preservation for 1-2 hours, continuously heating at 800-950 degrees C, carrying out heat preservation for 1-2 hours, and slowly cooling to 25-35 degrees C to obtain pre-carbonized product; and (3) mixing the pre-carbonized product obtained in step (2) with activating agent, where the weight ratio of pre-carbonized product and activating agent is 1:(1-5), then placing in tubular furnace under nitrogen atmosphere condition, heating at 500 degrees C, keeping the temperature for 1-2 hours, continuously heating at 800-1000 degrees C, maintaining the temperature for 1-2 hours, and slowly cooling to room temperature to obtain P.rubra substance graphene, where the activating agent is potassium hydroxide, aluminum nitrate and/or zinc nitrate.